Search Results (116)

The climate impact of Arctic aerosols, like the Arctic Haze, and their origin are not fully understood. Therefore, long-term aerosol observations in the Arctic are performed. In this study, we present a homogenised data set from a sun and star photometer operated in the European Arctic, in Ny-Ålesund, Svalbard, of the 20 years from 2004–2023. Due to polar day and polar night, it is crucial to use observations of both instruments. Their data is evaluated in the same way and follows the cloud-screening procedure of AERONET. Additionally, an improved method for the calibration of the star photometer is presented. We found out, that autumn and winter are generally more polluted and have larger particles than summer. While the monthly median Aerosol Optical Depth (AOD) decreases in spring, the AOD increases significantly in autumn. A clear signal of large particles during the Arctic Haze can not be distinguished from large aerosols in winter. With autocorrelation analysis, we found that AOD events usually occur with a duration of several hours. We also compared AOD events with large-scale processes, like large-scale oscillation patterns, sea ice, weather conditions, or wildfires in the Northern Hemisphere but did not find one single cause that clearly determines the Arctic AOD. Therefore the observed optical depth is a superposition of different aerosol sources. Full article

This study identifies the characteristics of water regions with negative normalized water-leaving radiance (nLw(λ)) values in the satellite observations of the Second-generation Global Imager (SGLI) sensor aboard the Global Change Observation Mission–Climate (GCOM-C) satellite. SGLI Level-2 data, along with atmospheric and in-water optical properties measured by the sun photometers in the AErosol RObotic NETwork-Ocean Color (AERONET-OC) from 26 sites globally, are utilized in this study. The focus is particularly on Tokyo Bay and the Ariake Sea, semi-enclosed water regions in Japan where previous research has pointed out the occurrence of negative nLw(λ) values due to atmospheric correction with SGLI. The study examines the temporal changes in atmospheric and in-water optical properties in these two regions, and identifies the characteristics of regions prone to negative nLw(λ) values due to atmospheric correction by comparing the optical properties of these regions with those of 24 other AERONET-OC sites. The time series results of nLw(λ) and the single-scattering albedo (ω(λ)) obtained by the sun photometers at the two sites in Tokyo Bay and Ariake Sea, along with SGLI nLw(λ), indicate the occurrence of negative values in SGLI nLw(λ) in blue band regions, which are mainly attributed to the inflow of absorptive aerosols. However, these negative values are not entirely explained by ω(λ) at 443 nm alone. Additionally, a comparison of in situ nLw(λ) measurements in Tokyo Bay and the Ariake Sea with nLw(λ) values obtained from 24 other AERONET-OC sites, as well as the inherent optical properties (IOPs) estimated through the Quasi-Analytical Algorithm version 5 (QAA_v5), identified five sites—Gulf of Riga, Long Island Sound, Lake Vanern, the Tokyo Bay, and Ariake Sea—as regions where negative nLw(λ) values are more likely to occur. These regions also tend to have lower nLw(λ) values at shorter wavelengths. Furthermore, relatively high light absorption by phytoplankton and colored dissolved organic matter, plus non-algal particles, was confirmed in these regions. This occurs because atmospheric correction processing excessively subtracts aerosol light scattering due to the influence of aerosol absorption, increasing the probability of the occurrence of negative nLw(λ) values. Based on the analysis of atmospheric and in-water optical measurements derived from AERONET-OC in this study, it was found that negative nLw(λ) values due to atmospheric correction are more likely to occur in water regions characterized by both the presence of absorptive aerosols in the atmosphere and high light absorption by in-water substances. Full article

The pandemic lockdown of the year 2020 has been generally accompanied by an improvement in the air quality. Here, we report data on the effects of lockdown limitations on the air quality in the metropolitan area of Naples (Italy) by following the evolution of main atmospheric pollutants over a five-year period and comparing their concentrations in the pandemic year 2020 with the previous (2018 and 2019) and following (2021 and 2022) two years. In particular, NO₂ and PM10 concentrations registered by representative air quality sampling station network and the columnar features of the aerosol characterized by a sun-photometer are considered. To avoid the possible influence of Saharan dust transport, which generally affects the observational area, the analysis has been limited to the days free from such events. Our findings evidence a tendency towards pre-pandemic conditions, notwithstanding some differences related to partial and temporary restrictions imposed even in the year 2021. For both near-surface NO₂ and PM, the observations confirm a significant reduction induced by the lockdown in 2020, besides the seasonal changes, and a gradual tendency towards more typical values in the following years. Also, the columnar aerosol data clearly highlight a gradual recovery of typical conditions in 2021 and 2022, confirming a peculiar effect of the pandemic lockdown of the year 2020 on the atmospheric aerosol characteristics that evidences a striking predominance of the fine component. Full article

The detection and evaluation of biomass burning and dust events are critical for understanding their impact on air quality, climate, and human health, particularly in the Mediterranean region. This research pioneers an innovative methodology that uses Sentinel-2 multispectral (MS) imagery to meticulously pinpoint and analyze long-transport dust outbreaks and biomass burning phenomena, originating both locally and transported from remote areas. We developed the dust/biomass burning (DBB) composite normalized differential index, a tool that identifies clear, dusty, and biomass burning scenarios in the selected region. The DBB index jointly employs specific Sentinel-2 bands: B2-B3-B4 for visible light analysis, and B11 and B12 for short-wave infrared (SWIR), exploiting the specificity of each wavelength to assess the presence of different aerosols. A key feature of the DBB index is its normalization by the surface reflectance of the scene, which ensures independence from the underlying texture, such as streets and buildings, for urban areas. The differentiation involves the comparison of the top-of-atmosphere (TOA) reflectance values from aerosol events with those from clear-sky reference images, thereby constituting a sort of calibration. The index is tailored for urban settings, where Sentinel-2 imagery provides a decametric spatial resolution and revisit time of 5 days. The average values of DBB achieve a 96% match with the coarse-mode aerosol optical depths (AOD), measured by a local station of the AERONET network of sun-photometers. In future studies, the map of DBB could be integrated with that achieved from Sentinel-3 images, which offer similar spectral bands, albeit with much less fine spatial resolution, yet benefit from daily coverage. Full article

The accuracy of cosmic ray observations by the Large High Altitude Air Shower Observatory Wide Field-of-View Cherenkov/Fluorescence Telescope Array (LHAASO-WFCTA) is influenced by variations in aerosols in the atmosphere. The solar photometer (CE318-T) is extensively utilized within the Aerosol Robotic Network as a highly precise and reliable instrument for aerosol measurements. With this CE318-T 23, 254 sets of valid data samples over 394 days from October 2020 to October 2022 at the LHAASO site were obtained. Data analysis revealed that the baseline Aerosol Optical Depth (AOD) and Ångström Exponent (AE) at 440–870 nm (AE_440–870nm) of the aerosols were calculated to be 0.03 and 1.07, respectively, suggesting that the LHAASO site is among the most pristine regions on Earth. The seasonality of the mean AOD is in the order of spring > summer > autumn = winter. The monthly average maximum of AOD_440nm occurred in April (0.11 ± 0.05) and the minimum was in December (0.03 ± 0.01). The monthly average of AE_440–870nm exhibited slight variations. The seasonal characterization of aerosol types indicated that background aerosol predominated in autumn and winter, which is the optimal period for the absolute calibration of the WFCTA. Additionally, the diurnal daytime variations of AOD and AE across the four seasons are presented. Our analysis also indicates that the potential origins of aerosol over the LHAASO in four seasons were different and the atmospheric aerosols with higher AOD probably originate mainly from Northern Myanmar and Northeast India regions. These results are presented for the first time, providing a detailed analysis of aerosol seasonality and origins, which have not been thoroughly documented before in this region, also enriching the valuable materials on aerosol observation in the Hengduan Mountains and Tibetan Plateau. Full article

Integrated systems are facing complex and changing environments with the wide application of atmospheric LiDAR in civil, aerospace, and military fields. Traditional analysis methods employ optical software to evaluate the optical performance of integrated systems, and cannot comprehensively consider the influence of optical and mechanical coupling on the optical performance of the integrated system, resulting in the unsatisfactory accuracy of the analysis results. Optical–mechanical integration technology provides a promising solution to this problem. A small-field-of-view LiDAR system with high repetition frequency, low energy, and single-photon detection technology was taken as an example in this study, and the Zernike polynomial fitting algorithm was programmed to enable transmission between optical and mechanical data. Optical–mechanical integration technology was employed to obtain the optical parameters of the integrated system under a gravity load in the process of designing the optical–mechanical structure of the integrated system. The experimental validation results revealed that the optical–mechanical integration analysis of the divergence angle of the transmission unit resulted in an error of 2.586%. The focal length of the telescope increased by 89 μm, its field of view was 244 μrad, and the error of the detector target surface spot was 4.196%. The continuous day/night detection results showed that the system could accurately detect the temporal and spatial variations in clouds and aerosols. The inverted optical depths were experimentally compared with those obtained using a solar photometer. The average optical depth was 0.314, as detected using LiDAR, and 0.329, as detected by the sun photometer, with an average detection error of 4.559%. Therefore, optical–mechanical integration analysis can effectively improve the stability of the structure of highly integrated and complex optical systems. Full article

A rare event of mixed biomass-burning and polluted dust aerosols was observed over Athens, Greece (37.9° N, 23.6° E), during 21–26 May 2014. This event was studied using a synergy of a 6-wavelength elastic-Raman-depolarization lidar measurements, a CIMEL sun photometer, and in situ instrumentation. The FLEXPART dispersion model was used to identify the aerosol sources and quantify the contribution of dust and black carbon particles to the mass concentration. The identified air masses were found to originate from Kazakhstan and Saharan deserts, under a rare atmospheric pressure system. The lidar ratio (LR) values retrieved from the Raman lidar ranged within 25–89 sr (355 nm) and 35–70 sr (532 nm). The particle linear depolarization ratio (δ_aer) ranged from 7 to 28% (532 nm), indicating mixing of dust with biomass-burning particles. The aerosol optical depth (AOD) values derived from the lidar ranged from 0.09–0.43 (355 nm) to 0.07–0.25 (532 nm). An inversion algorithm was used to derive the mean aerosol microphysical properties (mean effective radius (r_eff), single scattering albedo (SSA), and mean complex refractive index (m)) inside selected atmospheric layers. We found that r_eff was 0.12–0.51 (±0.04) µm, SSA was 0.94–0.98 (±0.19) (at 532 nm), while m ranged between 1.39 (±0.05) + 0.002 (±0.001)i and 1.63 (±0.05) + 0.008 (±0.004)i. The polarization lidar photometer networking (POLIPHON) algorithm was used to estimate the vertical profile of the mass concentration for the dust and non-dust components. A mean mass concentration of 15 ± 5 μg m⁻³ and 80 ± 29 μg m⁻³ for smoke and dust was estimated for selected days, respectively. Finally, the retrieved aerosol microphysical properties were compared with column-integrated sun photometer CIMEL data with good agreement. Full article

In the summer of 2017, huge wildfires in the British Columbia region (Canada) led to the injection of a remarkably high concentration of biomass burning aerosol in the atmosphere. These aerosol masses reached the city of Naples, Italy, at the end of August 2017, where they were characterized by means of a multiwavelength lidar and a sun–sky–lunar photometer. Here we report on the optical and microphysical properties of this aerosol in an intriguing condition, occurring on 4 September 2017, which is characterized by an interesting multi-layered vertical distribution of the aerosol. The Lidar profiles highlighted the presence of four aerosol layers, with two located in the lower troposphere and the other two at stratospheric altitudes. A rather thorough characterization of the biomass burning aerosol was carried out. The aerosol depolarization ratio showed an increasing dependence on the altitude with averaged values of 2–4% for the tropospheric layers, which are indicative of almost spherical smoke particles, and larger values in the stratospheric layers, suggestive of aspheric particles. Lidar-derived size distributions were retrieved for the first three aerosol layers, highlighting a higher particle concentration in the fine-mode fraction for the layers observed at higher altitudes. A dominance of fine particles in the atmosphere (fine-mode fraction > 0.8) with low absorption properties (absorption AOD < 0.0025 and SSA > 0.97) was also observed over the whole atmospheric column by sun photometer data. The space-resolved results provided by the lidar data are consistent with the columnar features retrieved by the AERONET sun photometer, thus evidencing the reliability and capability of lidar characterization of atmospheric aerosol in a very interesting condition of multiple aerosol layers originating from Canadian fires overpassing the observation station. Full article

The radiative budget is one of the key factors that influences climate change. The aim of this study was to analyze the radiative regime in Moscow using the RAD-MSU(BSRN) complex and to estimate the radiative effects of the main geophysical factors during the 2021–2023 period. This complex is equipped and maintained according to the recommendations of the Baseline Surface Radiation Network; however, it is not a part of this network. In cloudless conditions, the decrease in global shortwave irradiance (Q) is about 18–22% due to the aerosol content with a pronounced change in the direct to diffuse ratio. In winter, the increase in Q is about 45 W/m² (or 9%) at h = 30° due to a high surface albedo and reduced aerosol and water vapor contents, while the net shortwave irradiance (Bsh) demonstrates a significant decrease due to the prevailing effects of snow albedo. In cloudy conditions, a nonlinear dependence of Q and Bsh cloud transmittance on the relative sunshine duration is observed. The mean changes in Q for the 2021–2023 against the 1955–2020 period are characterized by negative anomalies (−22%) in winter and positive anomalies in summer (+3%) due to the changes in cloudiness. This is in line with the global tendencies in the long-term changes in shortwave irradiance in moderate climates in Europe in recent years. Full article

Aerosols play a crucial role in the surface radiative budget by absorbing and scattering both shortwave and longwave radiation. While most aerosol types exhibit a relatively minor longwave radiative forcing when compared to their shortwave counterparts, dust aerosols stand out for their substantial longwave radiative forcing. In this study, radiometers, a sun photometer, a microwave radiometer and the parameterization scheme for clear-sky radiation estimation were integrated to investigate the radiative properties of aerosols. During an event in Xianghe, North China Plain, from 25 April to 27 April 2018, both the composition (anthropogenic aerosol and dust) and the aerosol optical depth (AOD, ranging from 0.3 to 1.5) changed considerably. A notable shortwave aerosol radiative effect (SARE) was revealed by the integrated system (reaching its peak at −131.27 W·m⁻² on 26 April 2018), which was primarily attributed to a reduction in direct irradiance caused by anthropogenic aerosols. The SARE became relatively consistent over the three days as the AODs approached similar levels. Conversely, the longwave aerosol radiative effect (LARE) on the dust days ranged from 8.94 to 32.93 W·m⁻², significantly surpassing the values measured during the days of anthropogenic aerosol pollution, which ranged from 0.35 to 28.67 W·m⁻², despite lower AOD values. The LARE increased with a higher AOD and a lower Ångström exponent (AE), with a lower AE having a more pronounced impact on the LARE than a higher AOD. It was estimated that, on a daily basis, the LARE will offset approximately 25% of the SARE during dust events and during periods of heavy anthropogenic pollution. Full article

A sun photometer is a type of photometer that points at the sun, and it has been playing an increasingly important role in characterizing aerosols across the world. As long as the solar photometer is accurately calibrated, the optical thickness of the aerosol can be obtained from the measured value of this device. When the calibration of a single instrument is not accurate, the inversion quantity varies greatly. The calibration constant of the sun photometer changes during its use process; thus, calibrations are frequently needed in order to ensure the accuracy of the measured value. The calibration constant of the solar photometer is usually determined using the Langley method. Internationally, AERONET has two Langley calibration stations: the Mauna Loa observatory in the United States and the Izaña observatory in Spain. So far, the International Comparison and Calibration System has been established in Beijing, similar to AERONET at GSFC, but the Langley calibration system has not yet been established. Therefore, it is necessary to select a suitable calibration station in China. This paper studies the requirements of the calibration station using the Langley method. We used long-term records of satellite-derived measurements and survey data belonging to the aerosol optical thickness data of SNPP/VIIRS, CERES, MERRA-2, etc., in order to gain a better understanding of whether these stations are suitable for calibration. From the existing astronomical observation stations, meteorological stations, and the Sun–Sky Radiometer Observation Network (SONET) observation stations in China, the qualified stations were selected. According to the statistical data from the Ali observatory, the monthly average of clear sky is 20.21 days, and it is always greater than 15 days. The monthly average of aerosol is not more than 0.15 and is less than 0.3. We believe that the atmosphere above the Ali observatory is stable, and the results show that the Ali observatory has excellent weather conditions. This study can provide a selection of calibration sites for solar photometer calibrations in China that may need to be further characterized and evaluated, and at the same time provide a method to exclude unsuitable calibration sites. Full article

The versatile Generalized Retrieval of Aerosol and Surface Properties (GRASP) algorithm exploits the advantages of synergic ground-based aerosol observations such as radiometric (sensitive to columnar aerosol optical and microphysical properties) and lidar (sensitive to vertical distribution of the optical properties) observations. The synergy is possible when the complementary data is mutually constrained by GRASP parametrization that includes, for the first time ever, the degree of linear polarization (DoLP) parameter measured by a polarized sun-sky-lunar AERONET photometer (380, 440, 500, 675, 870, 1020, and 1640 nm) in synergy with the vertical profiles from an elastic lidar (355, 532, and 1064 nm). First, a series of numerical tests is performed using simulated data generated using a climatology of data and ground-based measurements. The inversions are performed with and without random noise for five different combinations of input data, starting from the AERONET-like dataset and increasing to the complex one by adding more information for three aerosol scenarios: I—high aerosol optical depth (AOD) with dominant coarse mode; II—low AOD with dominant coarse mode; III—high AOD with dominant fine mode. The inclusion of DoLP improves (i) the retrieval accuracy of the fine-mode properties when it is not dominant; (ii) the retrieval accuracy of the coarse-mode properties at longer wavelengths and that of the fine-mode properties at shorter wavelengths; (iii) the retrieval accuracy of the coarse-mode real part of the refractive index (up to 36% reduction), but has no effect on the retrieval of the imaginary part; (iv) reduces up to 83% the bias of the sphere fraction (SF) retrieval in coarse-mode dominated regimes; and (v) the root mean square error (RMSE) of the retrieval for most of the parameters in all scenarios. In addition, the addition of more photometer channels in synergy with a three-wavelength elastic lidar reduces the RMSE for the real part (67% in the coarse mode) and the imaginary part (35% in the fine mode) of the refractive index, the single scattering albedo (38% in the fine mode), the lidar ratio (20% in the coarse mode), and the SF (43%). Full article

To better understand aerosol vertical distribution and radiation effects, the seasonal variation and vertical distribution characteristics of aerosol optical properties were analyzed based on the aerosol extinction coefficient, depolarization ratio and backscatter Ångström exponent derived from the dual-wavelength polarization lidar at the Semi-Arid Climate and Environment Observatory of Lanzhou University (SACOL) from December 2009 to November 2012. Combining the CE-318 sun photometer, the microphysical, optical and vertical distribution characteristics of aerosol during a dust process were discussed comprehensively. The results revealed that the vertical profiles of the aerosol extinction coefficient and depolarization ratio clearly had seasonal variation characteristics. The aerosol optical depth (AOD) integrating with the aerosol extinction coefficient within 0–2 km in the spring, summer, autumn and winter accounted for 48%, 45%, 56% and 58% of the total AOD, respectively. The non-spherical feature was most distinctive in the spring, followed by the winter, autumn and summer. The particle size of aerosol in the lower layer was larger than that in the upper layer according to the vertical profile of the backscatter Ångström exponent. The cluster analysis of backward trajectory showed SACOL is dominated by dust aerosol in the spring and the mixtures of dust with anthropogenic pollution in the winter. A dust event in April 2010 was selected and the analysis showed that it mainly came from the high-altitude and long-range transportation from the Taklamakan Desert. During this period, the extinction coefficient increased up to 0.9 km⁻¹, the maximum AOD was 2.21 and the SSA ranged from 0.92 to 0.99. The radiation force in the atmosphere reached 126.15 W/m². It can be found that the influence of aerosol on the atmospheric radiation effect cannot be ignored. Full article

The sky-radiometer/sun-photometer is the most widely used instrument for obtaining aerosol optical depth (AOD) or aerosol optical properties worldwide. Due to the existence of field of view (FOV, 1°), the radiation received by the sky-radiometer includes the forward scattering in addition to direct solar irradiance. This leads to more diffuse light errors of retrieved AODs, especially for shorter wavelength and heavily polluted weather conditions. Using simulation data of three typical aerosol particles (dust, soot, water-soluble), we first verified the accuracy of the Monte Carlo method for calculating the forward scattering effect. Based on the sky-radiometer data collected in Xi’an (2015–2020) where heavy pollution weather is common, the relative errors and correction factors of the AOD were obtained under different conditions, including various short wavelengths (≤400 nm), solar zenith angles (SZAs) and AODs. Our analysis indicates the close dependence of AOD correction factors on wavelength, SZA, AOD and the optical properties of aerosol particles. The mean relative error in Xi’an increases with the decrease of wavelength (~16.1% at 315 nm) and decreases first and then increases with the increase of the SZA. The relative errors caused by forward scattering can exceed 10% when the AOD is greater than 1 and 25% when the AOD is larger than 2 in the ultraviolet (UV) band. The errors with a wavelength greater than 400 nm and an AOD below 1.0 can be within 5%, which can be ignored. The correlation coefficients of AODs before and after a correction from 315 nm to 400 nm are greater than 0.96, which basically increase with the increase of the wavelength. This indicates that the significance of the forward scattering effect in the Xi’an area with heavy pollution cannot be ignored for short wavelengths. However, such effect is negligible at the longer wavelengths and lower AODs (<1.0) of a sky-radiometer. Full article

Particulate matter (PM) is one of the major air pollutants that has adverse impacts on human health. The aim of this study is to present an alternative approach for retrieving fine PM (particles with an aerodynamic diameter less than 2.5 μm, PM_2.5) using artificial intelligence. Ground-based instruments, including a hand-held Microtops II sun photometer (for aerosol optical depth), a PurpleAir sensor (for PM_2.5), and Rotronic sensors (for temperature and relative humidity), are used for the machine learning algorithm training. The retrieved PM_2.5 reveals an adequate performance with an error of 0.08 μg m⁻³ and a Pearson correlation coefficient of 0.84. Full article